Global atmospheric black carbon inferred from AERONET

Publication Type  Journal Article
Year of Publication  2003
Authors  Sato, M.; Hansen, J.; Koch, D.; Lacis, A.; Ruedy, R.; Dubovik, O.; Holben, B.; Chin, M.; Novakov, T.
Journal Title  Proceedings of the National Academy of Sciences of the United States of America
Volume  100
Issue  11
Pages  6319-6324
Journal Date  May 27
ISBN Number  0027-8424
Accession Number  ISI:000183190700008
Key Words  aerosols; air pollution; climate change; single-scattering albedo; optical-properties; sulfate aerosols; light-absorption; variability; satellite; model; dust; sun
Abstract  

AERONET, a network of well calibrated sunphotometers, provides data on aerosol optical depth and absorption optical depth at >250 sites around the world. The spectral range of AERONET allows discrimination between constituents that absorb most strongly in the UV region, such as soil dust and organic carbon, and the more ubiquitously absorbing black carbon (BC). AERONET locations, primarily continental, are not representative of the global mean, but they can be used to calibrate global aerosol climatologies produced by tracer transport models. We find that the amount of BC in current climatologies must be increased by a factor of 2-4 to yield best agreement with AERONET, in the approximation in which BC is externally mixed with other aerosols. The inferred climate forcing by BC, regardless of whether it is internally or externally mixed, is approximate to1 W/m(2), most of which is probably anthropogenic. This positive forcing (warming) by BC must substantially counterbalance cooling by anthropogenic reflective aerosols. Thus, especially if reflective aerosols such as sulfates are reduced, it is important to reduce BC to minimize global warming.

Notes  

684DTTimes Cited:51Cited References Count:29

URL  <Go to ISI>://000183190700008
DOI  DOI 10.1073/pnas.0731897100